Adding a Gmail account
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Select Outlook > Preferences > Accounts.
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Click the plus (+) sign > New Account.
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Type your email address > Continue.
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Type your password > Add Account.
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Click Continue.
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Sign-in to your Gmail account within Outlook for Mac. This is for users who are on Build 16.15.18070902 and higher.
Have you already added your Gmail account to Outlook then see, Improved auth for existing Gmail users.
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Select an account to sign in.
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Type the account password.
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The Google account permissions window appears. Click Allow.
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Click Open Microsoft Outlook.
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Select Done to start using Outlook 2016 for Mac.